NATIONAL WATER QUALITY LABORATORY
                          TECHNICAL MEMORANDUM 97-02


                 ----RESPONSE REQUESTED BY JANUARY 1, 1997----


                                                     November 25, 1996

To:       Water Resources Division

From:     Peter F. Rogerson, Chief
          National Water Quality Laboratory
          Branch of Analytical Services

Subject:  Proposed Replacement or Elimination of NWQL Procedures

Authors:  Peter F. Rogerson, Chief, NWQL, (303)467-8003 (rogerson)

Revision: None

                               BACKGROUND

In the interests of efficiency and economy, the National Water Quality
Laboratory (NWQL) has reviewed all analytical tests performed at the NWQL
to determine which procedures could be eliminated, replaced, or contracted
to increase efficiency and save money for our customers.  Within this
Technical Memorandum are proposals to replace or eliminate several NWQL
analytical procedures.  This proposed action is not final.  Over the next
30 days, please examine these proposed changes for impact on your ongoing
projects.  If you find that these changes are unacceptable, please let me
know so that the NWQL can work with you to minimize the impact or to
maintain a critical procedure.  Following the 30-day comment period, the
NWQL will issue a technical memorandum with an effective date for the
changes.  Although I believe there will be no unacceptable changes in data
quality, I am encouraging all NWQL customers to verify this lack of
significant impact prior to implementing the proposed procedure.

Thank you for working with us to provide the best possible analytical
service at the lowest possible price.

                                 SCOPE

The Inorganic Chemistry Program used the following criteria to set
priorities for analytical tests that could be eliminated, replaced, or
contracted:

1.  Small numbers of submitted samples.
2.  Small numbers of customers submitting samples.
3.  Availability of similar tests from NWQL or other sources such as
    contract labs.
4.  Analytical procedures that are particularly difficult to set up.
5.  Analytical procedures on which the NWQL appears to be losing money.

The NWQL proposes to eliminate the following Low-Level [Low-Ionic Strength
(LIS)] tests and replace them with the equivalent regular level tests:
     
    [LIS, low-ionic strength; GFAA, graphite furnace atomic absorption; 
    ICP/MS, inductively coupled plasma/mass spectrometry; DCP, direct-
    current plasma; ICP, inductively coupled plasma; AA, atomic absorption]

NAME               LAB CODE*   PARAMETER   REPLACE WITH            LAB CODE 
                                 CODE                            (PARAM. CODE)
-------------------------------------------------------------------------------
Acidity, LIS        1266      71825 B     Acidity, Regular       1 (71825 A)

Alkalinity, LIS     1270      90410 B     Alkalinity, Regular   70 (90410 A)

Manganese, LIS,     1257      01056 D     Manganese, ICP/MS   1793 (01056 G)
  GFAA              

Nickel, LIS, GFAA   1256      01065 D     Nickel, GFAA or     1562 (01065 F) or
                                          ICP/MS              1795 (01065 G)

Cobalt, LIS, GFAA   1252      01035 E     Cobalt, GFAA or     1556 (01035 F) or
                                          ICP/MS              1890 (01035 G)

Cadmium, LIS, GFAA  1250      01025 E     Cadmium, GFAA or    1554 (01025 F) or
                                          ICP/MS              1788 (01025 G)

Lead, LIS, GFAA     1254      01049 E     Lead, GFAA or       1560 (01049 F) or
                                          ICP/MS              1792 (01049 G)

Copper, LIS, GFAA   1253      01040 E     Copper, GFAA or     1558 (01040 F) or
                                          ICP/MS              1791 (01040 G)

Chromium, LIS, GFAA 1251      01030 D     Chromium, GFAA or   1936 (01030 I) or
                                          ICP/MS              1789 (01030 G)

Zinc, LIS, GFAA     1276      01090 D     Zinc, ICP or ICP/MS  671 (01090 B) or
                                                              1798 (01090 G)

Aluminum, LIS, DCP  1267      01106 D     Aluminum, ICP or    2111 (01106 F) or
                                          ICP/MS              1784 (01106 G)

Calcium, LIS, ICP   1273      00915 B     Calcium, ICP         659 (00915 D)

Magnesium, LIS, AA   832      00925 A     Magnesium, ICP       663 (00925 C)

Magnesium, LIS, ICP 1274      00925 D     Magnesium, ICP       663 (00925 C)

Sodium, LIS, AA      834      00930 A     Sodium, ICP          675 (00930 C)

Sodium, LIS, ICP    1276      00930 D     Sodium, ICP          675 (00930 C)

Potassium, LIS, AA  0833      00935 A     Potassium, AA         54 (00935 B)

*The lab codes for the eliminated tests will become invalid.
-------------------------------------------------------------------------------
-------------------------------------------------------------------------------

Volatile Dissolved Solids will be eliminated because there have been no
requests for this test in over a year.  There are insufficient requests to
justify maintaining the Volatile Bottom Material Solids test; therefore, it
will be offered only as a custom method and priced according to the cost of
setup and analysis.  NWQL analyzed only 60 samples for total Nitrogen by
Antek during 1994.  In contrast, many thousands of samples were analyzed by
Kjeldahl Nitrogen, on both filtered and unfiltered water.  Therefore, NWQL
plans to discontinue total Nitrogen by Antek and only offer Kjeldahl
Nitrogen.  The following three tests will be eliminated:

     [ROE, residue on evaporation; diss., dissolved; Vol., volatile; Btm.,
     bottom; TKN, Total Kjeldahl Nitrogen]

NAME              LAB CODE*   PARAMETER   REPLACE WITH            LAB CODE 
                                CODE                            (PARAM. CODE)
-------------------------------------------------------------------------------
Solids, ROE,         229      00520 A     Delete. No Requests.         -
Volatile, Diss.  

Solids, Vol.,        516      00496 A     Custom Analysis Only         -
Btm. Material 

Nitrogen, Antek     1570      00602 C     Nitrogen, TKN         1688 (00625 C)

*The lab codes for the eliminated tests will become invalid.
-------------------------------------------------------------------------------
-------------------------------------------------------------------------------

The following individual elemental determinations by atomic absorption
(AA) have already been replaced by more efficient multielement inductively
coupled plasma (ICP) techniques as announced in NWQL Technical Memorandum
96.04, effective April 1, 1996:

     [ICP, inductively coupled plasma; AA, atomic absorption; 
      mg/L, milligram/Liter]

NAME              LAB CODE*   PARAMETER   REPLACE WITH            LAB CODE 
                                CODE                            (PARAM. CODE)
-------------------------------------------------------------------------------
Barium,                7       01005 B    Barium,               641 (01005 C)
Filtered Water, AA                        Filtered Water, ICP

Beryllium,           170       01010 A    Beryllium,            655 (01010 B) 
Filtered Water, AA                        Filtered Water, ICP

Cadmium,             126       01025 A    Cadmium,              673 (01025 D)
Filtered Water, AA                        Filtered Water, ICP

Calcium,              12       00915 C    Calcium,              659 (00915 D) 
Filtered Water AA                         Filtered Water, ICP

Cobalt,              148       01035 A    Cobalt,               644 (01035 C)
Filtered Water, AA                        Filtered Water, ICP

Copper,              151       01040 A    Copper,               657 (01040 C)
Filtered Water, AA                        Filtered Water, ICP

Iron,                172       01046 C    Iron,                 645 (01046 D)
Filtered Water, AA                        Filtered Water, ICP

Lead,                191       01049 A    Lead,                 646 (01049 C)
Filtered Water, AA                        Filtered Water, ICP

Lithium,              39       01130 A    Lithium,              664 (01130 B)
Filtered Water, AA                        Filtered Water, ICP

Magnesium,            40       00925 B    Magnesium,            663 (00925 C)
Filtered Water, AA                        Filtered Water, ICP

Manganese,            42       01056 A    Manganese,            648 (01056 C)
Filtered Water, AA                        Filtered Water, ICP
 
Nickel,              197       01065 A    Nickel,               721 (01065 E)
Filtered Water, AA                        Filtered Water, ICP

Sodium,               59       00930 B    Sodium,              675 (00930 C)
Filtered Water, AA                        Filtered Water, ICP¹

Strontium,            62       01080 A    Strontium,           652 (01080 B) 
Filtered Water, AA                        Filtered Water, ICP
 
Zinc,                 67       01090 A    Zinc,                671 (01090 B)
Filtered Water, AA                        Filtered Water, ICP

*The lab codes for the replaced tests will become invalid.
¹Sodium by ICP is less sensitive than Sodium by AA (detection limits of 
 0.2 vs. 0.1 mg/L)
-------------------------------------------------------------------------------
-------------------------------------------------------------------------------

The NWQL has replaced the Direct Current Plasma (DCP) atomic emission
spectrometric determination of Aluminum (Al) and Boron (B) in filtered
water with an ICP determination as specified in NWQL Technical Memorandum
96.10.  The DCP lab codes for Al and B will become invalid.

The next table of tests will be available from a contract laboratory 
through the NWQL.  For information on how to submit samples to the contractor,
along with additional information such as sample batch size limitations,
please contact Bob Brock (RDBROCK) (303) 467-8097.  These tests are U.S.
Environmental Protection Agency (USEPA) methods that have been available
from the NWQL.  However, they have been requested infrequently, and it
is not economical to maintain them at NWQL.

NAME                         LAB CODE*     PARAMETER       REPLACE WITH
                                              CODE                            
-------------------------------------------------------------------------------
Cyanide, Bottom Material       1235         00721 B         Contract
Antimony, Bottom Material       534         01098 A         Contract
Barium, Bottom Material         521         01008 A         Contract
Beryllium, Bottom Material      522         01013 A         Contract
Molybdenum, Bottom Material     523         01063 A         Contract
Strontium, Bottom Material      530         01083 A         Contract
Calcium, Whole Water (USEPA)    324         00916 A         Contract
Magnesium, Whole Water (USEPA)  325         00927 A         Contract
Sodium, Whole Water (USEPA)     326         00929 A         Contract
Potassium, Whole Water (USEPA)  327         00937 A         Contract
Digestion, USEPA,               124      (preparation       Contract  
  for Ca, Mg, K, Na                     procedure only)

*The lab codes for these tests will become invalid.
-------------------------------------------------------------------------------
-------------------------------------------------------------------------------

The NWQL is now offering USEPA drinking-water methods for 47 organic and 14
inorganic constituents regulated by the State of Colorado.  These methods
comply with all USEPA drinking-water certification requirements and
constitute the NWQL USEPA-approved drinking-water determinations.  
Certification is performed by the State of Colorado and sanctioned by the 
USEPA, Region VIII.  An NWQL Technical Memorandum on this subject will be 
published.  If there is interest in using these drinking-water methods prior 
to the release of this memo, please contact Al Driscoll (DRISCOLL), 
(303) 467-8042.

The NWQL has substantial technical reservations about the tests for Sulfide
and for Hexavalent Chromium in water samples.  Both constituents are known to
be unstable, and USEPA-approved field-test kits are available from Hach 
Chemical.  The NWQL recommends that these constituents be determined onsite 
using the Hach field test.  NWQL will discontinue the following two tests as 
laboratory determinations:

NAME                      LAB CODE*   PARAMETER     REPLACE WITH
                                        CODE                            
------------------------------------------------------------------------------
Sulfide, Whole Water         89       00745 A       Field test:  Hach #8131

Chromium, Hexavalent,        16       01032 A       Field Test:  Hach #8023
Filtered Water 

*The lab codes for these discontinued tests will become invalid.
------------------------------------------------------------------------------
------------------------------------------------------------------------------

The Organic Chemistry Program at the NWQL also examined all analytical
tests to determine which could be eliminated, replaced, or sent to contract
laboratories.  These four tests have been requested fewer than 50 times in 
1993 and in 1994.  The detection limit for the existing USGS Oil and Grease 
in Bottom Material method is known to be too high for most purposes, and 
there is insufficient need to justify a more sensitive (and expensive) test. 
The two Inorganic Carbon methods involve substantial set-up costs when they 
are requested.  Because of the expense and the small number of requests, 
NWQL is discontinuing these tests and offering them only by contract.  The 
method for Tannin and Lignin had not been requested for several years but 
recently has been requested by one District hydrologist; this need is also 
being met by contract.

NAME                         LAB CODE*     PARAMETER       REPLACE WITH
                                             CODE                       
------------------------------------------------------------------------------
Oil & Grease, Bottom Material   531         00557 A        Contract

Carbon, Inorganic, Whole Water   19         00685 A        Contract

Carbon, Inorganic,              306         00691 A        Contract 
Filtered Water

Tannin and Lignin               138         32240 A        Contract

*The lab codes for these discontinued tests will become invalid.
------------------------------------------------------------------------------
------------------------------------------------------------------------------

The NWQL offers many schedules of pesticides in water that are typically
divided into classes of pesticides [organochlorine (OCs), organophosphate
(OPs), Atrazine-types, and carbamates] and combinations of classes.
Schedules are also offered for either whole-water or filtered water (total
or dissolved).  For some classes, such as carbamates, the pesticides reside
exclusively in the dissolved fraction because they have high solubilities,
but for two classes, OCs and OPs, the solubilities in water are low enough
that they will partition into the suspended particulate matter to a large
(and variable) extent.  The NWQL currently offers four filtered water
schedules of OC and OP pesticides and related compounds.  These four
schedules can recover different concentrations of analytes depending on the
amount of particulate matter present, the percent organic carbon on the
particles, and the partition coefficients of each analyte.  The NWQL offers
corresponding schedules for whole-water extractions that have better
recoveries of analytes.  The whole-water test is less expensive in all 
cases because the whole-water schedules do not require filtration.  
Current reporting limits are identical.  The NWQL proposes to eliminate the 
four filtered-water schedules and suggests that its customers use the 
corresponding whole-water schedule.  

The following table lists the four filtered-water schedules to be eliminated 
and the corresponding whole-water schedules that can be used in replacement.  
For complete information about these schedules, please see the NWQL 1995 
Services Catalog (OFR 95-352, p. 50-52).

Eliminate:                              Replace with:                        
Filtered water Schedule No.*            Whole water Schedule No.
------------------------------------------------------------------------------
Schedule 1316 (OPs)                     Schedule 1319 (OPs)                
Schedule 1321 (OCs)                     Schedule 1324 (OCs)                 
Schedule 1331 (OCs + OPs)               Schedule 1334 (OCs + OPs)           
Schedule 1361 (PCBs)                    Schedule 1364 (PCBs)                

*These filtered-water schedules will become invalid.
------------------------------------------------------------------------------
------------------------------------------------------------------------------

Finally, NWQL proposes to eliminate Schedule 1359 which measures eight
carbamate pesticides in whole-water samples.  These pesticides have high
water solubilities, so their concentrations are not expected to change
because of filtration.  Schedule 2050/2051 measures 41 similar pesticides
and metabolites in filtered water at much lower detection limits than measured 
by Schedule 1359.  Therefore, now that Schedule 2050/2051 has become a fully 
approved USGS analytical method, Schedule 1359 will be discontinued.  
Schedule 2050/2051 costs less than Schedule 1359, includes far more compounds, 
and has much lower detection limits.

Eliminate:                               Replace with:                     
---------------------------------------------------------------------------
Schedule 1359* (carbamates)              Schedule 2050/2051               

*This schedule will become invalid.
---------------------------------------------------------------------------
---------------------------------------------------------------------------

The Radiochemistry Unit has two analytical determinations to be eliminated
that have not been requested in several years and which have alternative
determinations.

NAME              LAB CODE*   PARAMETER   REPLACE WITH           LAB CODE 
                                CODE                           (PARAM. CODE)
-----------------------------------------------------------------------------
Radium-228 Filtered  850       81366 A    Radium-228 Filtered   1364 (81366 C)
Radon-222            490       82305 A    Radon-222             1369 (82330 B)

*The lab codes for these determinations will become invalid.
------------------------------------------------------------------------------
------------------------------------------------------------------------------

The replacement Radium-228 determination uses only 2 liters instead of 
7 liters of sample, has the same method detection limit (MDL) (1.0 pCi/L), 
and is approved by USEPA.  The replacement Radon-222 determination is less
expensive, is expected to be approved by USEPA, and provides results that
are available more quickly.  The Radon-222 test to be eliminated uses a
fragile, expensive bubbler system and provides lower detection limits than
most customers require.





Effect on Data Base:  There is no effect on existing data.
Supersedes:           None
Key Words:            Eliminate Procedures, Trace Metals, Solids, Nitrogen
                      Antek, Sulfide, Hexavalent Chromium, Oil and Grease, 
                      Carbon, Filtered, Pesticides, Carbamates, Radium-228,
                      Radon-222
Distribution:  Water Resources Division Distribution "E" plus the Netnews
               usgs.labnews & .water.quality; and 
               http://wwwnwql.cr.usgs.gov/